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The prior rules of designing Ti

Yingying Jian, Danyao Qu, Lihao Guo, Yujin Zhu, Chen Su, Huanran Feng, Guangjian Zhang, Jia Zhang, Weiwei Wu, Ming-Shui Yao

《化学科学与工程前沿（英文）》 2021年 第15卷 第3期   页码 505-517 doi: 10.1007/s11705-020-2013-y

摘要： Working temperature, sensitivity, and selectivity are some of the characteristics of the applied gas sensors. How to design and fabricate an ideal gas sensor working at room temperature is still challenging and attracting lots of interest. Two-dimensional (2D) materials with ultra-thin structure have been demonstrated as a family of ideal candidates to achieve this goal. Among them, Ti C T MXene, a kind of layered sheet synthesized by selectively etching MAX phases materials, shows remarkable potential to be the sensitive materials solely or in a composite. However, their designing rules are still lacking critical thinking from the viewpoint of the intrinsic property of Ti C T MXene based materials. In this article, two critical features, i.e., the thickness of the sensitive materials, and the scope of the analytes, are elaborated towards Ti C T MXene based gas sensors after characterizing the performance of sensing reducing gases (NH and CO) and oxidizing gas (NO ). First, the thinner the Ti C T MXene sensitive layer, the better the sensitivity. Second, the Ti C T MXene based gas sensor is not suitable for strong and moderate oxidation gas due to its ease of oxidation. These two rules are demonstrated, and could be considered with priority both in the future researches and practical applications.

关键词： MXene based sensor     prior     reducing gases     oxidizing gases    

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Overlooked nitrogen-cycling microorganisms in biological wastewater treatment

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1426-2

摘要：

• AOA and comammox bacteria can be more abundant and active than AOB/NOB at WWTPs.

关键词： Ammonia oxidizing archaea (AOA)     Complete ammonia oxidizing (comammox) bacteria     Dissimilatory nitrate reduction to ammonium (DNRA) bacteria     Nitrate/nitrite-dependent anaerobic methane oxidizing (NOx-DAMO) microorganisms     Engineering application    

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Enhancement on the ammonia oxidation capacity of ammonia-oxidizing archaeon originated from wastewater

《环境科学与工程前沿（英文）》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1375-1

摘要：

• AOA’s ammonia oxidizing capacity was enhanced under moderate magnetic field.

关键词： Ammonia-oxidizing archaeon     Ammonia oxidation     Magnetic field     Magnetotaxis     Heredity    

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Research progress and prospects of complete ammonia oxidizing bacteria in wastewater treatment

《环境科学与工程前沿（英文）》 2022年 第16卷 第9期 doi: 10.1007/s11783-022-1555-2

摘要：

• Comammox bacteria have unique physiological characteristics.

关键词： Complete ammonia oxidizing (comammox) bacteria     Nitrogen cycle     Physiological characteristics     Wastewater treatment    

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Systematical strategies for wastewater treatment and the generated wastes and greenhouse gases in China

Jingbo GUO, Fang MA, Yuanyuan QU, Ang LI, Liang WANG

《环境科学与工程前沿（英文）》 2012年 第6卷 第2期   页码 271-279 doi: 10.1007/s11783-011-0328-0

摘要： China now faces double challenges of water resources shortage and severe water pollution. To resolve Chinese water pollution problems and reduce its impacts on human health, economic growth and social development, the situation of wastewater treatment was investigated. Excess sludge and greenhouse gases (GHGs) emitted during wastewater treatment were also surveyed. It is concluded that Chinese water pollution problems should be systematically resolved with inclusion of wastewater and the solid waste and GHGs generated during wastewater treatment. Strategies proposed for the wastewater treatment in China herein were also adequate for other countries, especially for the developing countries with similar economic conditions to China.

关键词： wastewater treatment     solid waste     greenhouse gases     systematical strategies    

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Abundance and distribution of ammonia-oxidizing archaea in Tibetan and Yunnan plateau agricultural soils

Kun DING,Xianghua WEN,Liang CHEN,Daishi HUANG,Fan FEI,Yuyang LI

《环境科学与工程前沿（英文）》 2014年 第8卷 第5期   页码 693-702 doi: 10.1007/s11783-014-0635-3

摘要： As low oxygen and high ultraviolet (UV) exposure might significantly affect the microbial existence in plateau, it could lead to a specialized microbial community. To determine the abundance and distribution of ammonia-oxidizing archaea (AOA) in agricultural soil of plateau, seven soil samples were collected respectively from farmlands in Tibet and Yunnan cultivating the wheat, highland-barley, and colza, which are located at altitudes of 3200–3800 m above sea level. Quantitative PCR (q-PCR) and clone library targeting on gene were used to quantify the abundances of AOA and ammonia-oxidizing bacteria (AOB), and characterize the community structures of AOA in the samples. The number of AOA cells (9.34 × 10 –2.32 × 10 g soil) was 3.86–21.84 times greater than that of AOB cells (6.91 × 10 –1.24 × 10 g soil) in most of the samples, except a soil sample cultivating highland-barley with an AOA/AOB ratio of 0.90. Based Kendall’s correlation coefficient, no remarkable correlation between AOA abundance and the environmental factor was observed. Additionally, the diversities of AOA community were affected by total nitrogen and organic matter concentration in soils, suggesting that AOA was probably sensitive to several environmental factors, and could adjust its community structure to adapt to the environmental variation while maintaining its abundance.

关键词： ammonia-oxidizing archaea     ammonia-oxidizing bacteria     quantitative PCR     clone library     plateau    

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Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

《环境科学与工程前沿（英文）》 2022年 第16卷 第6期 doi: 10.1007/s11783-021-1506-3

摘要：

• The early corrosion process in the cast iron pipes was investigated.

关键词： Cast iron pipe corrosion     Drinking water distribution systems     Chlorine disinfection     Iron-oxidizing bacteria     Coupling effects    

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The impact of ultrasonic treatment on activity of ammonia-oxidizing bacteria and nitrite-oxidizing bacteria

Siqi Li, Min Zheng, Shuang Wu, Yu Xue, Yanchen Liu, Chengwen Wang, Xia Huang

《环境科学与工程前沿（英文）》 2019年 第13卷 第6期 doi: 10.1007/s11783-019-1166-8

摘要： • Conditions for ultrasonic treatment to achieve partial nitritation are optimized. • Ultrasound reduces metabolic activity and releases intracellular metabolites. • Mechanical shearing is essential to inhibit nitrite oxidation. The ultrasonic treatment of sludge has been considered as an effective method to facilitate the partial nitritation of municipal sewage. This study aims to reveal the effects of ultrasound on ammonia-oxidizing bacteria (AOB) and nitrite-oxidizing bacteria (NOB). The impact factors including ultrasonic irradiation time and intensity, sludge concentration, thermal effect and released free radicals were studied. The maximized difference between the changes in AOB and NOB activities were obtained with 10 g mixed liquor suspended solids (MLSS)/L, using 0.9 kJ/mL ultrasonic energy density and 12 h interval time. The increased ultrasonic intensity destroyed the floc structure of activated sludge, increased the microbial death, and decreased the cellular ATP level. Further, the mechanism exploration indicated that the mechanical shearing could be a critical factor in achieving the nitritation with inhibitory effect on nitrite oxidation.

关键词： Ultrasonic treatment     Optimal control     Nitrifying bacteria     Mechanism analysis    

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Community diversity and distribution of ammonia-oxidizing archaea in marsh wetlands in the black soil

Chunhong Chen, Hong Liang, Dawen Gao

《环境科学与工程前沿（英文）》 2019年 第13卷 第4期 doi: 10.1007/s11783-019-1146-z

摘要：

AOA amoA genes in the soils of the two wetlands affiliated with three lineages.

The main drivers of AOA community were pH and total organic carbon and ammonium.

The soil characteristics rather than the vegetation control the AOA community.

关键词： Ammonia-oxidizing archaea     amoA gene     Freshwater marsh     Diversity     Distribution    

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Applicability of the Arrhenius model for Ammonia Oxidizing Bacteria subjected to temperature time gradients

Alberto MANNUCCI,Giulio MUNZ,Gualtiero MORI,Claudio LUBELLO,Jan A. OLESZKIEWICZ

《环境科学与工程前沿（英文）》 2015年 第9卷 第6期   页码 988-994 doi: 10.1007/s11783-014-0751-0

摘要： The aim of this work is to identify the range of applicability of Arrhenius type temperature dependence for Ammonia Oxidizing Bacteria (AOB) subjected to temperature time gradients through continuous titrimetric tests. An innovative online differential titrimetric technique was used to continuously monitor the maximum biologic ammonia oxidation rate of the biomass selected in a pilot scale membrane bioreactor, as a function of temperature time gradients. The monitoring technique is based on the measurement of alkalinity and hydrogen peroxide consumption rates in two parallel reactors operated in non-limiting substrate conditions for AOB; both reactors were continuously fed with mixed liquor and in one of them AOB were inhibited with allylthiourea. The effects of temperature decrease rates in the range 1 to 4°C·h were evaluated by controlling the titrimetric reactor in the temperature range 10°C–20°C. The dependence of growth kinetics on temperature time gradients and the range of applicability of Arrhenius model for temperature dependency of AOB growth kinetics were assessed. The Arrhenius model was found to be accurate only with temperature gradients lower than 2°C·h . The estimated Arrhenius coefficients ( ) were shown to increase from 1.07 to 1.6 when the temperature decrease rate reached 4°C·h .

关键词： nitrification rate     temperature effect     continuous titrimetric tests     time-gradient temperature variations     Ammonia Oxidizing Bacteria (AOB)    

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Community dynamics of ammonia oxidizing bacteria in a full-scale wastewater treatment system with nitrification

Xiaohui WANG, Xianghua WEN, Hengjing YAN, Kun DING, Man HU

《环境科学与工程前沿（英文）》 2011年 第5卷 第1期   页码 92-98 doi: 10.1007/s11783-010-0254-6

摘要： To determine whether the functional stability of nitrification was correlated to a stable community structure of ammonia oxidizing bacteria (AOB) in a full-scale wastewater treatment plant, the AOB community dynamics in a wastewater treatment system was monitored over one year. The community dynamics were investigated using specific PCR followed by terminal restriction fragment length polymorphism (T-RFLP) analysis of the gene. The T-RFLP results indicated that during the period of nitrification stability, the AOB community structure in the full-scale wastewater treatment system was relatively stable, and the average change rate every 15 d of the system was 6.6%±5.8%. The phylogenetic analysis of the cloned gene showed clearly that the dominant AOB in the system was spp. The results of this study indicated that throughout the study period, the AOB community structure was relatively stable in the full-scale wastewater treatment system with functional stability of nitrification.

关键词： ammonia-oxidizing bacteria (AOB)     community dynamics     terminal restriction fragment length polymorphism (T-RFLP)     nitrification performance    

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Effects of hydraulic retention time on nitrification activities and population dynamics of a conventional activated sludge system

Hongyan LI, Yu ZHANG, Min YANG, Yoichi KAMAGATA

《环境科学与工程前沿（英文）》 2013年 第7卷 第1期   页码 43-48 doi: 10.1007/s11783-012-0397-8

摘要： The effects of hydraulic retention time (HRT) on the nitrification activities and population dynamics of a conventional activated sludge system fed with synthetic inorganic wastewater were investigated over a period of 260 days. When the HRT was gradually decreased from 30 to 5 h, the specific ammonium-oxidizing rates (SAOR) varied between 0.32 and 0.45 kg (kg mixed liquor suspended solids (MLSS)·d) , and the specific nitrate-forming rates (SNFR) increased from 0.11 to 0.50 kg (kg MLSS·d) , showing that the decrease in HRT led to a significant increase in the nitrite oxidation activity. According to fluorescence in situ hybridization (FISH) analysis results, the proportion of ammonia-oxidizing bacteria (AOBs) among the total bacteria decreased from 33% to 15% with the decrease in HRT, whereas the fraction of nitrite-oxidizing bacteria (NOBs), particularly the fast-growing sp., increased significantly (from 4% to 15% for NOBs and from 1.5% to 10.6% for sp.) with the decrease in HRT, which was in accordance with the changes in SNFR. A short HRT favored the relative growth of NOBs, particularly the fast-growing sp., in the conventional activated sludge system.

关键词： ammonia-oxidizing bacteria     hydraulic retention time     nitrification activity     nitrite-oxidizing bacteria     population dynamics    

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Stability of an annular viscous liquid jet in compressible gases with different properties inside and

Chunji YAN, Maozhao XIE,

《能源前沿（英文）》 2010年 第4卷 第2期   页码 198-204 doi: 10.1007/s11708-009-0054-5

摘要： A spatial linear instability analysis is conducted on an annular viscous liquid jet injected into compressible gases and a three-dimensional model of the jet is developed. The model takes into account differences between the velocities, densities of the gases inside and outside of the liquid jet. Theoretical analysis reveals that there exist 9 dimensionless parameters controlling the instability of the liquid jet. Numerical computations reveal some basic characteristics in the breakup and atomization process of the liquid jet as well as influences of these relevant parameters. Major observations and findings of this study are as follows. The Mach number plays a destabilizing role and the inner Mach number has a greater effect on the jet instability than the outer Mach number. The Reynolds number always tends to promote the instabilities of the liquid jet, but its influence is very limited. The Weber number and the gas-to-liquid density ratio also have unstable effects and can improve the atomization of liquid jets. Furthermore, the effects of the Weber number and gas-to-liquid density ratio on the maximum growth rates of axisymmetric and non-axisymmetric disturbances and corresponding dominant wave numbers are manifested in a linear way, while that of the Mach number is non-linear. The effect of Reynolds on the maximum growth rates is non-linear, but the dominant wavenumber is almost not affected by the Reynolds number.

关键词： liquid jet     dominant wave number     compressibility     instability    

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Effects of oxidizing environment on digestate humification and identification of substances governing

《环境科学与工程前沿（英文）》 2022年 第16卷 第8期 doi: 10.1007/s11783-022-1520-0

摘要：

• Liquid digestate humification was investigated under different oxidizing environment.

关键词： Liquid digestate     MnO2     Oxygen     DOM transformation     Humic-like acids    

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Microprofiles of activated sludge aggregates using microelectrodes in completely autotrophic nitrogen removal over nitrite (CANON) reactor

Yongtao LV,Xuan CHEN,Lei WANG,Kai JU,Xiaoqiang CHEN,Rui MIAO,Xudong WANG

《环境科学与工程前沿（英文）》 2016年 第10卷 第2期   页码 390-398 doi: 10.1007/s11783-015-0818-6

摘要： Microsensor measurements and fluorescence in situ hybridization (FISH) analysis were combined to investigate the microbial populations and activities in a laboratory-scale sequencing batch reactor (SBR) for completely autotrophic nitrogen removal over nitrite (CANON). Fed with synthetic wastewater rich in ammonia, the SBR removed 82.5±5.4% of influent nitrogen and a maximum nitrogen-removal rate of 0.52 kgN·m ·d was achieved. The FISH analysis revealed that aerobic ammonium-oxidizing bacteria (AerAOB) and anaerobic ammonium-oxidizing bacteria (AnAOB) dominated the community. To quantify the microbial activities inside the sludge aggregates, microprofiles were measured using pH, dissolved oxygen (DO), , and microelectrodes. In the outer layer of sludge aggregates (0–700 μm), nitrite-oxidizing bacteria (NOB) showed high activity with 4.1 μmol·cm ·h of maximum nitrate production rate under the condition of DO concentration higher than 3.3 mg·L . Maximum AerAOB activity was detected in the middle layer (depths around 1700 μm) where DO concentration was 1.1 mg·L . In the inner layer (2200–3500 μm), where DO concentration was below 0.9 mg·L , AnAOB activity was detected. We thus showed that information obtained from microscopic views can be helpful in optimizing the SBR performance.

关键词： microelectrodes     CANON     aerobic ammonium-oxidizing bacteria     anaerobic ammonium-oxidizing bacteria     nitrite-oxidizing bacteria    

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标题 作者 时间 类型 操作

The prior rules of designing Ti

Yingying Jian, Danyao Qu, Lihao Guo, Yujin Zhu, Chen Su, Huanran Feng, Guangjian Zhang, Jia Zhang, Weiwei Wu, Ming-Shui Yao

期刊论文

Overlooked nitrogen-cycling microorganisms in biological wastewater treatment

期刊论文

Enhancement on the ammonia oxidation capacity of ammonia-oxidizing archaeon originated from wastewater

期刊论文

Research progress and prospects of complete ammonia oxidizing bacteria in wastewater treatment

期刊论文

Systematical strategies for wastewater treatment and the generated wastes and greenhouse gases in China

Jingbo GUO, Fang MA, Yuanyuan QU, Ang LI, Liang WANG

期刊论文

Abundance and distribution of ammonia-oxidizing archaea in Tibetan and Yunnan plateau agricultural soils

Kun DING,Xianghua WEN,Liang CHEN,Daishi HUANG,Fan FEI,Yuyang LI

期刊论文

Synergistic effects of sodium hypochlorite disinfection and iron-oxidizing bacteria on early corrosion

期刊论文

The impact of ultrasonic treatment on activity of ammonia-oxidizing bacteria and nitrite-oxidizing bacteria

Siqi Li, Min Zheng, Shuang Wu, Yu Xue, Yanchen Liu, Chengwen Wang, Xia Huang

期刊论文

Community diversity and distribution of ammonia-oxidizing archaea in marsh wetlands in the black soil

Chunhong Chen, Hong Liang, Dawen Gao

期刊论文

Applicability of the Arrhenius model for Ammonia Oxidizing Bacteria subjected to temperature time gradients

Alberto MANNUCCI,Giulio MUNZ,Gualtiero MORI,Claudio LUBELLO,Jan A. OLESZKIEWICZ

期刊论文

Community dynamics of ammonia oxidizing bacteria in a full-scale wastewater treatment system with nitrification

Xiaohui WANG, Xianghua WEN, Hengjing YAN, Kun DING, Man HU

期刊论文

Effects of hydraulic retention time on nitrification activities and population dynamics of a conventional activated sludge system

Hongyan LI, Yu ZHANG, Min YANG, Yoichi KAMAGATA

期刊论文

Stability of an annular viscous liquid jet in compressible gases with different properties inside and

Chunji YAN, Maozhao XIE,

期刊论文

Effects of oxidizing environment on digestate humification and identification of substances governing

期刊论文

Microprofiles of activated sludge aggregates using microelectrodes in completely autotrophic nitrogen removal over nitrite (CANON) reactor

Yongtao LV,Xuan CHEN,Lei WANG,Kai JU,Xiaoqiang CHEN,Rui MIAO,Xudong WANG

期刊论文